The formation ages and tectonic features of the Bulunkuole Complex (BKC) is critical for understanding the geological evolution of the western section of the West Kunlun Orogenic Belt (WKOB), and they are also critical for understanding the metallogenic background of the Taxkorgan Iron Belt. In this paper, we report new geochemical and in situ zircon U-Pb isotopes data for the most southwestern iron-bearing formation of the BKC. The petrography and sedimentation ages of the BKC reveal that the main part of the BKC was emplaced in the Early to Late Cambrian period as a giant accretionary wedge formed during the Proto-Tethys Ocean south-southwestward subduction. The high-pressure metamorphic rocks located at the margin of the Kangxiwa Fault should be further disintegrated from the Cambrian BKC to form a Triassic accretionary complex. Geochemical characteristics indicate that the metasedimentary rocks of the Cambrian BKC derived predominantly from the regional contemporary intermediate to felsic source rocks, and deposited in the fore-arc basin. Provenance studies further demonstrate that the detrital materials were mainly sourced from the Gondwana-affinity terranes, Mazar Terrane as well as the volcanic and magmatic rocks produced during the Tethys subduction. The metamorphism of the Cambrian BKC occurred at ca. 200 Ma in the western section of the WKOB. Proto-Tethys Ocean did not close until 230 Ma, possibly during the Early Mesozoic (200-180 Ma).

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