Forests are important compartments influencing the environmental fate of persistent organic pollutants (POPs). To illustrate the effect of forests on the regional cycle of POPs, a level IV fugacity fate and transport model coupled with a detailed dynamic-forest module was applied to simulate the long-term variations of PCB-153 in China, where forest coverage accounts for approximately one fifth of land area. In the scenarios with forests, atmospheric outflow from China was 69% of that in the scenario without forests due to the enhanced storage in soil, degradation, and leaching. Previous studies regarded high-latitude areas, such as the polar region and boreal forests, as environments capable of reducing mobility of PCB-153, and they act as sinks of POPs. This modeling result suggests that tropical and subtropical forests may also play a similar role despite high temperatures favoring volatilization. Unlike boreal forest, the low-latitude forests may reduce the overall lifetime of PCB-153 in China due to enhanced degradation in warmer and moist soils of the tropical and subtropical area. Given that approximately half of the global forests are located in tropical and subtropical regions, they can be important environments influencing the global geochemical cycle and distribution of POPs, hence deserving more scientific attention by modeling and empirical studies.(c) 2021 Elsevier B.V. All rights reserved.
Publication name |
SCIENCE OF THE TOTAL ENVIRONMENT Volume: 778 Article Number: 146285 DOI: 10.1016/j.scitotenv.2021.146285 Published: JUL 15 2021 |
Author(s) |
Xu, Yue; Tian, Chongguo; Nizzetto, Luca; Zhang, Gan |
Corresponding author(s) |
XU Yue xu-yue@mail.gyig.ac.cn Chinese Acad Sci, Inst Geochem, State Key Lab Environm Geochem, Guiyang 550002, Peoples R China. | View here for the details
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